论文标题

压电响应力显微镜中的动态操作:创建具有较大机电响应的非平衡阶段

Dynamic manipulation in piezoresponse force microscopy: creating non-equilibrium phases with large electromechanical response

论文作者

Kelley, Kyle P., Ren, Yao, Morozovska, Anna N., Eliseev, Eugene A., Ehara, Yoshitaka, Funakubo, Hiroshi, Giamarchi, Thierry, Balke, Nina, Vasudevan, Rama K., Cao, Ye, Jesse, Stephen, Kalinin, Sergei V.

论文摘要

铁电材料中的域墙壁和拓扑缺陷已成为功能性电子设备(包括内存和逻辑)功能性电子设备的强大新范式。同样,壁相互作用和动态基础是从巨型机电反应到记忆效应的广泛的中尺度现象。探索各个领域壁的功能,它们的相互作用以及对域结构的受控修改对于应用和基本物理研究至关重要。然而,这些特征的动态性质严重限制了其本地物理的研究,因为在压电响应力显微镜中应用局部偏见或压力会诱导壁移作为主要反应。在这里,我们介绍了一种基于自动化实验控制和修改域结构的新方法,从而使用实际空间基于图像的反馈来控制铁电开关期间的尖端偏置,从而使修改路线在域下方的域状态下进行调节。为探索域壁动力学和具有较大机电响应的亚稳态的探索,证明了这种自动实验方法。

Domains walls and topological defects in ferroelectric materials have emerged as a powerful new paradigm for functional electronic devices including memory and logic. Similarly, wall interactions and dynamics underpin a broad range of mesoscale phenomena ranging from giant electromechanical responses to memory effects. Exploring the functionalities of individual domain walls, their interactions, and controlled modifications of the domain structures is crucial for applications and fundamental physical studies. However, the dynamic nature of these features severely limits studies of their local physics since application of local biases or pressures in piezoresponse force microscopy induce wall displacement as a primary response. Here, we introduce a fundamentally new approach for the control and modification of domain structures based on automated experimentation whereby real space image-based feedback is used to control the tip bias during ferroelectric switching, allowing for modification routes conditioned on domain states under the tip. This automated experiment approach is demonstrated for the exploration of domain wall dynamics and creation of metastable phases with large electromechanical response.

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