论文标题

活性棕色颗粒聚集体在多孔壁上的形态学转变

Morphological transitions of active Brownian particle aggregates on porous walls

论文作者

Das, Suchismita, Chelakkot, Raghunath

论文摘要

活动性布朗颗粒(ABP)的运动诱导的壁聚集是一种良好的现象。在这里,我们研究了ABP在多孔壁上的聚集,这使颗粒可以在大运动中穿透。我们表明,活性聚集体经历了从连接的致密相物到断开的液滴的形态学转变,壁孔隙度和颗粒自动动力的增加,类似于平衡流体中的润湿透明跃迁。我们表明,在形态学上不同的状态都是稳定的,并且至少在某些参数区域与初始条件无关。我们的分析表明,壁孔隙度的变化会影响聚集体的内在特性,并改变有效的壁凝集界面张力,与形态过渡的外观一致。因此,对密度以及取向分布的密切分析表明,这种形态过渡的根本原因不一定针对具有多孔壁的系统,并且可以通过对限制壁的特性调整较大的限制性,活性系统进行观察。

Motility-induced wall aggregation of active Brownian particles (ABPs) is a well-studied phenomenon. Here, we study the aggregation of ABPs on porous walls, which allows the particles to penetrate through at large motility. We show that the active aggregates undergo a morphological transition from a connected dense-phase to disconnected droplets with an increase in wall porosity and the particle self-motility, similar to wetting-dewetting transitions in equilibrium fluids. We show that both morphologically distinct states are stable, and independent of initial conditions at least in some parameter regions. Our analysis reveals that changes in wall porosity affect the intrinsic properties of the aggregates and changes the effective wall-aggregate interfacial tension, consistent with the appearance of the morphological transition. Accordingly, a close analysis of the density, as well as orientational distribution, indicates that the underlying reason for such morphological transitions is not necessarily specific to the systems with porous walls, and it can be possible to observe in a larger class of confined, active systems by tuning the properties of confining walls.

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