论文标题
拓扑结构剂的光学响应 - 与探针电场相互作用的Quantum-Dot Hybrid
Optical response of a topological-insulator--quantum-dot hybrid interacting with a probe electric field
论文作者
论文摘要
我们研究拓扑绝缘子纳米颗粒与受施加电场的量子点之间的相互作用。拓扑绝缘子的电磁响应是从绝对近似中的轴支电动力学得出的。局部模式按偶极骨模式进行量化,该模式将偶极性伴侣与量子点偶联在一起。因此,我们将混合动力车视为与单个骨模式相互作用的两级系统,其中耦合强度编码有关纳米颗粒非平凡拓扑的信息。混合体与环境的相互作用是通过与辐射输出模式的连续库和声子模式的储层实现的。特别是,我们使用Zubarev的绿色函数的方法来得出系统的光吸收光谱的表达式。我们将结果应用于一个现实的系统,该系统由由Tlbise $ _ {2} $制成的拓扑绝缘子纳米颗粒与硒化量子点相互作用,两者都沉浸在聚合物层中,例如聚(甲基甲基丙烯酸甲酯)。光吸收光谱表现出具有线条形状的FANO共振,这在很大程度上取决于电场的极化以及拓扑磁性极化性$θ$。我们的结果和方法也可以应用于非复杂磁电材料,例如cr $ _ {2} $ o $ $ _ {3} $。
We study the interaction between a topological insulator nanoparticle and a quantum dot subject to an applied electric field. The electromagnetic response of the topological insulator is derived from axion electrodynamics in the quasistatic approximation. Localized modes are quantized in terms of dipolar bosonic modes, which couples dipolarly to the quantum dot. Hence, we treat the hybrid as a two-level system interacting with a single bosonic mode, where the coupling strength encodes the information concerning the nontrivial topology of the nanoparticle. The interaction of the hybrid with the environment is implemented through the coupling with a continuum reservoir of radiative output modes and a reservoir of phonon modes. In particular, we use the method of Zubarev's Green functions to derive an expression for the optical absorption spectrum of the system. We apply our results to a realistic system which consists of a topological insulator nanoparticle made of TlBiSe$_{2}$ interacting with a cadmium selenide quantum dot, both immersed in a polymer layer such as poly(methyl methacrylate). The optical absorption spectrum exhibits Fano resonances with a line shape that strongly depends on the polarization of the electric field as well as on the topological magnetoelectric polarizability $θ$. Our results and methods can also be applied to nontopological magnetoelectric materials such as Cr$_{2}$O$_{3}$.