论文标题
WSE2的低温载体传输机制和光电导率
Low temperature carrier transport mechanism and photoconductivity of WSe2
论文作者
论文摘要
这项工作报道了杜松子钨(WSE2)薄膜中的电运输和温度依赖性光电导率。电导率分析表明,存在温度变化的三个区域。在较低的温度(<190k)下,由于Mott Hopping机制,载体将载体定位于电影中的小区域。中部区域(190至273 K)遵循SETO参数,并获得了低屏障高度(0.0873 eV),可能是改善载流子迁移率的原因。在较高的温度(> 273K)区域,热激活传导以〜138 MeV和98 MeV的两个激活能为主导。在光致发光分析中获得的峰归因于中频态的存在或缺陷状态,这些状态在WSE2的光导率中起重要作用。瞬态光电导率测量表现出一致的温度依赖性行为。还讨论了光强度和波长变化对WSE2薄膜光电导率的影响。光电流为1.19*10-5 a在125 K时,在350 K时,观察到3.12*10-4 A.轻on/OFF电流周期表明,电流可以恢复到其初始状态,该状态指向其稳定且出色的可逆性,WSE2薄膜设备在光电电视机应用中使用。
This work reports the electrical transport and temperature-dependent photoconductivity in tungsten diselenide (WSe2) thin films. The electrical conductivity analysis shows the presence of the three regions with temperature variation. At lower temperatures (<190K), carriers become localized to small regions in the film due to the Mott hopping mechanism. The middle region (190 to 273 K) follows Seto parameters and obtained low barrier height (0.0873 eV) may be responsible for the improved carrier mobility. At higher temperature (>273K) region, thermally activated conduction is dominated with two activation energies of ~138 meV and 98 meV. The peaks obtained in photoluminescent analysis attributes to the presence of mid-bandgap states or defect states which play an important role in the photoconductivity of WSe2. The transient photoconductivity measurements show consistent temperature-dependent behaviour. The effect of light intensity and wavelength variation on the photoconductivity of WSe2 thin films is also discussed. The photocurrent is 1.19*10-5 A at 125 K while at 350 K it was observed to be 3.12*10-4 A. The light-on/off current cycles show that the current can recover to its initial state which points to the stable and outstanding reversible properties of the WSe2 thin film device to be used in photodetector applications.