论文标题
莫特绝缘子在时间与频域中的光学区分性
Optical Distinguishability of Mott Insulators in Time vs Frequency Domain
论文作者
论文摘要
高谐波产生(HHG)有望提供对超快动态的见解,自发现以来,就一直处于Attosecond物理的最前沿。一类证明HHG的材料是Mott绝缘子,其电子性质引起了极大相关的性质。在这里,我们使用半填充的费米 - 哈伯德模型Mott绝缘子的范式表示,研究使用HHG响应来区分这些材料的潜力。我们根据Schrodinger方程对Magnus扩展对进化的近似的近似,这表明Mott绝缘子作为晶格间距,$ a $和驾驶场的强度,$ f_0 $,相对于频率增加,$ f_0 $增加。然后,通过对不同系统的数值模拟以及随后在时间和频域中对其响应进行比较来加强该参数。最终,当无量纲参数$ g \ equiv af_0 /ω_0$很大时,我们证明了两个域中Mott绝缘子的分辨率减少,尽管时间域提供了更高的区分性。导体免于这些趋势,在高$ g $的频域中变得更加区分。
High Harmonic Generation (HHG) promises to provide insight into ultrafast dynamics and has been at the forefront of attosecond physics since its discovery. One class of materials that demonstrate HHG are Mott insulators whose electronic properties are of great interest given their strongly-correlated nature. Here, we use the paradigmatic representation of Mott insulators, the half-filled Fermi-Hubbard model, to investigate the potential of using HHG response to distinguish these materials. We develop an analytical argument based on the Magnus expansion approximation to evolution by the Schrodinger equation that indicates decreased distinguishability of Mott insulators as lattice spacing, $a$, and the strength of the driving field, $F_0$, increase relative to the frequency, $ω_0$. This argument is then bolstered through numerical simulations of different systems and subsequent comparison of their responses in both the time and frequency domain. Ultimately, we demonstrate reduced resolution of Mott insulators in both domains when the dimensionless parameter $g \equiv aF_0 / ω_0$ is large, though the time domain provides higher distinguishability. Conductors are exempted from these trends, becoming much more distinguishable in the frequency domain at high $g$.