论文标题

熵驱动的顺序以纳米磁铁数组

Entropy-driven order in an array of nanomagnets

论文作者

Saglam, Hilal, Duzgun, Ayhan, Kargioti, Aikaterini, Harle, Nikhil, Zhang, Xiaoyu, Bingham, Nicholas S., Lao, Yuyang, Gilbert, Ian, Sklenar, Joseph, Watts, Justin D., Ramberger, Justin, Bromley, Daniel, Chopdekar, Rajesh V., O'Brien, Liam, Leighton, Chris, Nisoli, Cristiano, Schiffer, Peter

论文摘要

远程顺序通常与熵减少有关。但是,在某些特殊情况下,熵的增加也可以驱动。我们证明,单域纳米磁体的人造自旋冰阵列可以设计成熵驱动的顺序。我们专注于人造自旋冰结构,这是一个高度沮丧的阵列几何形状,具有零点的保里熵,该结构是通过在规范的方形冰晶格上选择性地创建常规空缺来形成的。我们通过实验和模拟探测热活跃的人造旋转冰冰层,测量单个纳米磁体的磁矩。我们在这些力矩的一个子集中发现了二维磁有序,我们证明,在矩的另一个子集中,我们证明了这是由无序诱导的(即增加熵)。与其他熵驱动的系统相反,俄罗斯方块人工旋转冰中的离散自由度是二进制的,在微观上都是可设计的,可以直接观察到,并且在模拟中可以精确地计算系统的熵。在此示例中,系统的相互作用和基态熵是明确的,它扩展了实验局势,以研究熵驱动的订单。

Long-range ordering is typically associated with a decrease in entropy. Yet, it can also be driven by increasing entropy in certain special cases. We demonstrate that artificial spin ice arrays of single-domain nanomagnets can be designed to produce entropy-driven order. We focus on the tetris artificial spin ice structure, a highly frustrated array geometry with a zero-point Pauli entropy, which is formed by selectively creating regular vacancies on the canonical square ice lattice. We probe thermally active tetris artificial spin ice both experimentally and through simulations, measuring the magnetic moments of the individual nanomagnets. We find two-dimensional magnetic ordering in one subset of these moments, which we demonstrate to be induced by disorder (i.e., increased entropy) in another subset of the moments. In contrast with other entropy-driven systems, the discrete degrees of freedom in tetris artificial spin ice are binary and are both designable and directly observable at the microscale, and the entropy of the system is precisely calculable in simulations. This example, in which the system's interactions and ground state entropy are well-defined, expands the experimental landscape for the study of entropy-driven ordering.

扫码加入交流群

加入微信交流群

微信交流群二维码

扫码加入学术交流群,获取更多资源