论文标题

在带宽控制的Mott Transition附近的有机导体中相干重载体

Coherent heavy charge carriers in an organic conductor near the bandwidth-controlled Mott transition

论文作者

Oberbauer, Sebastian, Erkenov, Shamil, Biberacher, Werner, Kushch, Natalia D., Gross, Rudolf, Kartsovnik, Mark V.

论文摘要

在过去的几十年中,莫特金属绝缘体过渡(MIT)的物理学引起了极大的兴趣。但是,尽管做出了广泛的努力,但一些关键的理论预测仍缺乏实验性确认。特别是,尚不清楚大型连贯的费米表面是否可以立即与带宽控制的一阶MIT生存。还缺少对准粒子有效质量的预测行为的定量实验验证,并通过多体相互作用重新归一化。在这里,我们通过使用有机$κ$ -Type盐作为示例性的准二维带宽控制的莫特绝缘子来解决这些问题,并通过磁量子振荡直接获得其电荷载体性能。我们追踪有效回旋质量的演变,因为通过精确控制的外部压力将传导带宽非常接近MIT。我们发现,质量重新归一化对带宽的微小变化的敏感性明显高于理论上的预测,并且在进入金属和绝缘相共存的过渡区域时,甚至进一步增强了。另一方面,即使在其稳定性的边缘,金属基态也可以保留大型连贯的费米表面,没有显着增强散射。

The physics of the Mott metal-insulator transition (MIT) has attracted huge interest in the last decades. However, despite broad efforts, some key theoretical predictions are still lacking experimental confirmation. In particular, it is not clear whether the large coherent Fermi surface survives in immediate proximity to the bandwidth-controlled first-order MIT. A quantitative experimental verification of the predicted behavior of the quasiparticle effective mass, renormalized by many-body interactions, is also missing. Here we address these issues by employing organic $κ$-type salts as exemplary quasi-two-dimensional bandwidth-controlled Mott insulators and gaining direct access to their charge carrier properties via magnetic quantum oscillations. We trace the evolution of the effective cyclotron mass as the conduction bandwidth is tuned very close to the MIT by means of precisely controlled external pressure. We find that the sensitivity of the mass renormalization to tiny changes of the bandwidth is significantly stronger than theoretically predicted and is even further enhanced upon entering the transition region where the metallic and insulating phases coexist. On the other hand, even at its very edge of stability the metallic ground state preserves a large coherent Fermi surface with no significant enhancement of scattering.

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