论文标题

在二氧化钒的名义磁磁性绝缘状态下低温下的自旋塞贝克效应

Spin Seebeck effect at low temperatures in the nominally paramagnetic insulating state of vanadium dioxide

论文作者

Luo, Renjie, Zhao, Xuanhan, Chen, Liyang, Legvold, Tanner J., Navarro, Henry, Schuller, Ivan K., Natelson, Douglas

论文摘要

二氧化钒的低温单斜层,绝缘阶段通常被认为是非磁性的,二聚钒原子形成了自旋单重,尽管在低温下可以看到顺磁反应。我们在VO2膜中发现了一个非局部自旋Seebeck信号,该信号出现在30 K以下,并且随温度降低而增加。旋转Seebeck响应对平面外部磁场具有非滞后依赖性。通过先前关于顺磁性自旋seebeck效应的效应和单斜基基态的预期磁激励的发现,讨论了这种顺磁性自旋seebeck响应。

The low temperature monoclinic, insulating phase of vanadium dioxide is ordinarily considered nonmagnetic, with dimerized vanadium atoms forming spin singlets, though paramagnetic response is seen at low temperatures. We find a nonlocal spin Seebeck signal in VO2 films that appears below 30 K and which increases with decreasing temperature. The spin Seebeck response has a non-hysteretic dependence on in-plane external magnetic field. This paramagnetic spin Seebeck response is discussed in terms of prior findings on paramagnetic spin Seebeck effects and expected magnetic excitations of the monoclinic ground state.

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