论文标题

BI2O2SE纳米线呈现高迁移率和强旋转轨道耦合

Bi2O2Se nanowires presenting high mobility and strong spin-orbit coupling

论文作者

Zhao, Kui, Liu, Huaiyuan, Tan, Congwei, Xiao, Jianfei, Shen, Jie, Liu, Guangtong, Peng, Hailin, Lu, Li, Qu, Fanming

论文摘要

在高质量的BI2O2SE纳米线上进行了系统的电运输特征,以说明其巨大的运输特性和Spintronics中的进一步应用潜力。通过化学蒸气沉积法合成的BI2O2SE纳米线提出了高达1.34*104 CM2V-1S-1的高场效应迁移率,并在下部后门面电压(VG)状态下表现出弹道传输,观察到电导率plateaus。当通过增加VG来进一步增加电子密度时,我们进入了相干状态和弱抗钙化(WAL)。发现从WAL提取的自旋松弛长度可调节,范围从〜100 nm至〜250 nm不等,并且比二维对应物(薄片)达到更强的自旋粘合耦合(SOC)。我们将强SOC和栅极可调性归因于表面积累层的存在,该层在表面上引起了强反转不对称。这种情况得到了观察到两个shubnikov-de Haas振荡频率的支持,它们对应于两种类型的载体,一种在地面上,另一个在散装中。具有高机动性和强大SOC的高质量的BI2O2SE纳米线可以在未来的Spintronics中起到非常前瞻性的作用。

Systematic electrical transport characterizations were performed on high-quality Bi2O2Se nanowires to illustrate its great transport properties and further application potentials in spintronics. Bi2O2Se nanowires synthesized by chemical vapor deposition method presented a high field-effect mobility up to 1.34*104 cm2V-1s-1, and exhibited ballistic transport in the low back-gate voltage (Vg) regime where conductance plateaus were observed. When further increasing the electron density by increasing Vg, we entered the phase coherent regime and weak antilocalization (WAL) was observed. The spin relaxation length extracted from the WAL was found to be gate tunable, ranging from ~100 nm to ~250 nm and reaching a stronger spin-obit coupling (SOC) than the two-dimensional counterpart (flakes). We attribute the strong SOC and the gate tunability to the presence of a surface accumulation layer which induces a strong inversion asymmetry on the surface. Such scenario was supported by the observation of two Shubnikov-de Haas oscillation frequencies that correspond to two types of carriers, one on the surface, and the other in the bulk. The high-quality Bi2O2Se nanowires with a high mobility and a strong SOC can act as a very prospective material in future spintronics.

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