论文标题

在填充的skutterudite化合物laru $ _4 $中,多绘制超导率AS $ _ {12} $由Muon Spin Rotation探测

Multigap Superconductivity in the Filled-Skutterudite Compound LaRu$_4$As$_{12}$ probed by muon spin rotation

论文作者

Bhattacharyya, A., Adroja, D. T., Koza, M. M., Tsutsui, S., Cichorek, T., Hillier, A. D.

论文摘要

MUON自旋旋转($μ$ SR)和非弹性X射线散射(IXS)用于研究填充的skutterudite化合物Laru $ _ {4} $的超导性能为$ _ {12} $。两间隙各向同性($ S+S $) - 波模型可以解释超流体密度的温度依赖性。零字段$μ$ SR的测量结果证实,进入超导状态后,时间反转对称不会破裂。在2、20和300 K处的晶格动力学的测量显示了声子模式的温度依赖性,这些温度依赖性在冷却时严格遵循的声子频率在准谐波图片中的预期状态下,声子频率的变化。 20〜K数据而不是标志着大多数声子频率的转折点。实际上,观察到从上方接近20〜k的硬化,而对于一些分支,在进一步冷却至2〜k时可以看到弱的软化。整个布里渊区的声子模式的观察到的分散关系与DFT预测匹配。我们的结果指出,Cutic Laru $ _ {4} $作为$ _ {12} $是研究多播超导性的良好参考材料,包括那些具有较低晶体学对称性(例如基于铁砷的超导体)的材料。

Muon spin rotation ($μ$SR) and inelastic X-ray scattering (IXS) were used to investigate the superconducting properties of the filled-skutterudite compound LaRu$_{4}$As$_{12}$. A two-gap isotropic ($s+s$)-wave model can explain the temperature dependence of the superfluid density. Zero field $μ$SR measurements confirm that the time-reversal symmetry does not break upon entering the superconducting state. The measurements of lattice dynamics at 2, 20 and 300 K revealed temperature dependencies of the phonon modes that do not follow strictly a hardening of phonon frequencies upon cooling as expected within the quasi-harmonic picture. The 20~K data rather mark a turning point for the majority of the phonon frequencies. Indeed a hardening is observed approaching 20~K from above, while for a few branches a weak softening is visible upon further cooling to 2~K. The observed dispersion relations of phonon modes throughout the Brillouin zone matches with the DFT prediction quite closely. Our results point out that cubic LaRu$_{4}$As$_{12}$ is a good reference material for studying multiband superconductivity, including those with lower crystallographic symmetries such as iron arsenide-based superconductors.

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