论文标题
整体纳米线激光表征是最佳设计的途径
Holistic nanowire laser characterization as a route to optimal design
论文作者
论文摘要
纳米线激光器可用于近场和片上光子应用,因为它们提供了可集成,相干和单色辐射。因此,波长尺度的纳米线既充当激光动作的增益介质和空腔:功能性能(阈值和波长)因此取决于每个纳米线的光电极和晶体学特性。但是,可扩展的自下而上的制造技术通常会遭受纳米间差异的差异,从而导致单个纳米线之间的产量和性能差异通常很大。建立制造控制,几何和材料特性与激光性能之间的关系是朝着优化的关键步骤,但是,由于此类特性的复杂相互依存关系,实现实验的挑战。在这里,我们提出了一种高通量相关方法,可以表征超过5000个单独的GAASP/GAAS多个量子井纳米线激光器。拟合自发发射的阈值载体密度可提供阈值,而相干长度测量值测量了终端的反射率。我们表明,由于量子限制和带填充效应,激光波长和阈值与单个量子井的宽度本质上相关。出乎意料的是,激光腔的特性(方形反射率和分布损失)与阈值之间没有很强的关系:相反,阈值与载体的非辐射重组寿命呈负相关。因此,这种方法提供了一种优化策略,该策略无法通过小规模研究来访问。量子井的质量和宽度限制了这些纳米线激光器的阈值,而不是腔质量。
Nanowire lasers are sought for near-field and on-chip photonic applications as they provide integrable, coherent and monochromatic radiation. A wavelength-scale nanowire acts as both the gain medium and the cavity for the lasing action: the functional performance (threshold and wavelength) is therefore dependent on both the opto-electronic and crystallographic properties of each nanowire. However, scalable bottom-up manufacturing techniques often suffer from inter-nanowire variation, leading to, often dramatic, differences in yield and performance between individual nanowires. Establishing the relationship between manufacturing controls, geometric and material properties and the lasing performance is a crucial step towards optimisation, however, this is challenging to achieve experimentally due to the complex interdependance of such properties. Here, we present a high-throughput correlative approach to characterise over 5000 individual GaAsP/GaAs multiple quantum well nanowire lasers. Fitting the spontaneous emission provides the threshold carrier density, while coherence length measurements measures end-facet reflectivity. We show that the lasing wavelength and threshold are intrinsically related to the width of a single quantum well due to quantum confinement and bandfilling effects. Unexpectedly, there is no strong relationship between the properties of the lasing cavity (facet reflectivity and distributed losses) and the threshold: instead the threshold is negatively correlated with the non-radiative recombination lifetime of the carriers. This approach therefore provides an optimisation strategy that is not accessible through small-scale studies. The quality and width of the quantum wells limit the threshold of these nanowire lasers, rather than the cavity quality.